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If shooter in general:
1. Oddworld: Stranger's Wrath
2. Max Payne

If only FPS:
1. Outlaws
2. The Operative: No One Lives Forever
Favorite on GOG: Deus Ex.

Favorite not on GOG: NOLF 1 & 2
"Reads the thread's title." OK:
https://www.youtube.com/watch?v=Z59AnkxekfI

"Reads the first post." Oh, right.

My favourite here: The Ultimate Doom

One that I would like most here: Turok 2: Seeds of Evil
Serious Sam

NOLF 1 & 2
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Grargar: "Reads the thread's title." OK:
https://www.youtube.com/watch?v=Z59AnkxekfI

"Reads the first post." Oh, right.
Yes! That was the line I had in my head when I wrote the title. You are the first person to catch it, well done old chap.
1. Serious Sam probably (but there's a few)

2. Soldier of Fortune
Zandronum Doom servers!
Well, Freddi Fish 2 (AMAZING first-person section; easy to learn, difficult to master) is sorely lacking from the catalogue here, but programs like Doom, Serious Sam, and Painkiller are decent ways to pass the time while waiting for the TRUE gem of fps to descend from heaven (or hell depending on where Retroism is based).
If it was still on GOG I'd say Descent, but since it's not...

1. Star Wars: Dark Forces
2. Tron 2.0
Praise the gods: Quake 3

Curse the IP laws: Soldier of Fortune (Raven, 2000)
1. Realms of the Haunting, or if you want a more "pure" FPS, Eradicator
2. Heretic. Haven't played it yet and so would love to see it here.
1. Star Wars Jedi Knight: Dark Forces II
2. Area 51 (2005)
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Elmofongo: Well regarding the my must have list of Importan/Classic/Popular Old School PC games which I have categorized the ones that are FPSes:

Bohemia Library (Thus includes Arma games)
Half-Life 1 and 2
Counter Strike and Condition Zero
Doom 3 and Ressurection of Evil expansion
Battlefield 1942, Vietnam, 2, and 2142
Call of Duty 1+United Offensive
SWAT 4
Hexen series
Heretic Games
Marathon series
Tom Clancy's Rainbow Six 2 and 3 and their expansions
Brother's in Arms Road to Hill 30 and Earned in Blood
Tron 2.0
Red Orchestra 1
Crysis 1+Warhead
No One Lives Forever 1 and 2
Medal of Honor: Pacific Assault
Duke Nukem games

Out of all the ones there the one I want the most is:

(Drum roll)

Crysis 1+ the Warhead stand-alone expansion.
A very good list, my friend. I agree with almost all of them. It would be nice if GOG were a little quicker in fulfilling requests.
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Stooner: 1. Serious Sam probably (but there's a few)

2. Soldier of Fortune
Ahh yes, Soldier of Fortune! I would particularly like to see SoF2 on GOG.
Post edited June 16, 2016 by VanCrusty