cogadh: The X-Men Legends comparison is a fair one and if you liked that game, you will probably thoroughly enjoy Freedom Force. However, just be aware that FF is far more "point and clicky" than XML and its descendants are, so don't expect the same kind of controls with the FF games.
Aaah, excellent. It is highly likely that this shall be my next GoG aquisition, then.
Thanks everyone for the help so far!
On a related note, can anyone recommend similar games I might enjoy? Deep character customization is a plus, while uber-large party sizes aren't so much, since I would prefer a small cast of characters I can keep a close eye on (no more than five in play and maybe twenty total) over lots of characters that overwhelm my obsessive need for even levelling.
EDIT: On an aside, I'm really considering three games at the moment -- MotoRacer 2, Stonekeep, and Freedom Force. This will make my 40th game, so I want it to be something a little special.